Issue 14, 2023

Advancing towards ready-to-use solid oxide fuel cells: 5 minute cold start-up with high-power performance

Abstract

The development of low-temperature solid oxide fuel cells (LT-SOFCs) as a mobile power source is attracting attention; however, limited understanding of rapid LT-SOFC operation constrains their use. Here, we present a high-performance LT-SOFC system capable of rapid thermal cycling and cold start-up, akin to ready-to-use. To achieve a ready-to-use LT-SOFC system, we modified a compact compressive sealing architecture implemented with a stacked disc spring, and a rapid thermal cycling with cold start-up was realized using a lamp heater. This LT-SOFC system reached target temperatures within 5 min of start-up and immediately exhibited an open-circuit potential of 1.124 V and a maximum power density of 1.123 W cm−2 at 600 °C. We evaluated this system with harsh thermal cycling (25–500 or 600 °C) for 3000 min and confirmed its degradation behavior in perovskite phase separation and interfacial delamination. Our results provide another breakthrough in LT-SOFC development for mobile applications.

Graphical abstract: Advancing towards ready-to-use solid oxide fuel cells: 5 minute cold start-up with high-power performance

Supplementary files

Article information

Article type
Communication
Submitted
22 Nov 2022
Accepted
18 Mar 2023
First published
27 Mar 2023

J. Mater. Chem. A, 2023,11, 7415-7421

Advancing towards ready-to-use solid oxide fuel cells: 5 minute cold start-up with high-power performance

H. Jeong, C. Lee, J. Son, S. Y. Lee, K. J. Yoon, D. Shin, M. Choi, S. S. Shin and H. Kim, J. Mater. Chem. A, 2023, 11, 7415 DOI: 10.1039/D2TA09092A

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